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Correlation between solvation structure and ion-conductive behavior of concentrated poly(ethylene carbonate)-based electrolytes. Molecular crowding electrolytes for high-voltage aqueous batteries. Formation and stability of celluloseвЂ“copperвЂ“NaOH crystalline complex. Crystalline Cellulose and Derivatives 1st edn (Springer-Verlag, 2008). Ion conductivity through TEMPO-mediated oxidated and periodate oxidated cellulose membranes. Cellulose-based flexible functional materials for emerging intelligent electronics. Pure cellulose lithium-ion battery separator with tunable pore size and improved working stability by cellulose nanofibrils. High-performance all-solid-state batteries enabled by salt bonding to perovskite in poly(ethylene oxide). Ultrathin, flexible, solid polymer composite electrolyte enabled with aligned nanoporous host for lithium batteries. Improved lithium ionic conductivity in composite polymer electrolytes with oxide-ion conducting nanowires. Nanocomposite polymer electrolytes and their impact on the lithium battery technology. Single lithium-ion conducting polymer electrolytes based on a super-delocalized polyanion. Single-ion BAB triblock copolymers as highly efficient electrolytes for lithium-metal batteries. Hybrid electrolytes with controlled network structures for lithium metal batteries. Crosslinked poly(tetrahydrofuran) as a loosely coordinating polymer electrolyte. Suppression of lithium dendrite growth using cross-linked polyethylene/poly(ethylene oxide) electrolytes: a new approach for practical lithium-metal polymer batteries. Poly(ethylene oxide)-based electrolytes for lithium-ion batteries. Promising routes to a high Li + transference number electrolyte for lithium ion batteries. Solid-state electrolytes for lithium-ion batteries: fundamentals, challenges and perspectives. Designing polymers for advanced battery chemistries. Lithium battery chemistries enabled by solid-state electrolytes. Nanocomposite polymer electrolytes for lithium batteries. Ionic conductivity in crystalline polymer electrolytes.

Polymer electrolytes for lithium polymer batteries. Nonaqueous liquid electrolytes for lithium-based rechargeable batteries. Furthermore, we have verified the universality of this molecular-channel engineering approach with other polymers and cations, achieving similarly high conductivities, with implications that could go beyond safe, high-performance solid-state batteries. This one-dimensional ion conductor also allows ion percolation in thick LiFePO 4 solid-state cathodes for application in batteries with a high energy density.

In addition to high Li + conductivity (1.5В Г—В 10 в€’3 siemens per centimetre at room temperatureВ along the molecular chainВ direction), the Cu 2+-coordinated cellulose ion conductor also exhibits a high transference number (0.78, compared with 0.2вЂ“0.5 in other polymers 2) and a wide window of electrochemical stability (0вЂ“4.5 volts) that can accommodate both the Li-metal anode and high-voltage cathodes. Through the coordination of copper ions (Cu 2+) with one-dimensional cellulose nanofibrils, we show that the opening of molecular channels within the normally ion-insulating cellulose enables rapid transport of Li + ions along the polymer chains.

Here we report a general strategy for achieving high-performance solid polymer ion conductors by engineering of molecular channels. Conversely, polymer ion conductors that are Li-metal-stable usually provide better interfacial compatibility and mechanical tolerance, but typically suffer from inferior ionic conductivity owing to the coupling of the ion transport with the motion of the polymer chains 1, 2, 3. Inorganic ion conductors allow fast ion transport, but their rigid and brittle nature prevents good interfacial contact with electrodes. Nature volumeВ 598, pages 590вЂ“596 ( 2021) Cite this articleДЄlthough solid-state lithium (Li)-metal batteries promise both high energy density and safety, existing solid ion conductors fail to satisfy the rigorous requirements of battery operations. Copper-coordinated cellulose ion conductors for solid-state batteries

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